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Next: Conclusions Up: Tunnelling through two dots Previous: Ohmic conductance

Current characteristics

 

The current-voltage characteristics have been calculated in figure 10 for a double dot system with specifications as indicated in the caption. Figure 11 shows the results for a system where the dot specifications have been swapped. Physically this simply amounts to varying the chemical potential in the right reservoir instead of the left reservoir.

At low temperatures two periods may be observed in the I-V characteristics. The larger period is given by the Coulomb repulsion in the first dot plus a single particle spacing tex2html_wrap_inline1442. The smaller period is simply given by the single particle spacing tex2html_wrap_inline1444. This behaviour is reminiscent of the current through a single dot with tex2html_wrap_inline1290 (see section iii). In other words, the second dot with its surrounding barriers acts as a single barrier with a reduced transparency. The electrons which have entered the first dot will tunnel into a lower energy level in the second dot at a rate of approximately tex2html_wrap_inline1418 since the levels in the dots will not normally line up. At larger temperatures the current curves will lose some features due to thermal smearing. This is clearly the case in figure 11.

However, the current curve of figure 10 has a more complicated form at high temperatures. It has a region of negative differential conductance which occurs in the bias range where the average occupancy of the first dot increases from one to two electrons with respect to the average occupation number at zero bias. This can be explained by considering the (unlikely) case where a pair of energy levels matches up for a given set of occupation numbers. This will result in a highly increased tunnelling rate between the dots. When the bias across the device is raised the average occupancy of the dot will increase. This means that the dots are less likely to contain the number of electrons for which the levels lined up. Consequently the tunnelling rate between the dots and hence the overall current will decrease, in spite of the fact that the total number of tunnelling paths is likely to have increased.

The temperature at which negative differential conductance can occur (if at all) is set by the energy difference of the matching pair of levels in the dots. Their energy separation has to be significantly less than tex2html_wrap_inline1450 for the tunnelling rate to increase dramatically. A higher temperature can cause some levels to match up which could not really be considered energetically close at lower temperatures. However, a higher temperature also means that there is a smaller probability that the total inter-dot tunnelling is dominated by just a single pair of levels. This will reduce the effect. The conclusion is that negative differential conductance is more likely to occur at higher temperatures, but when it occurs at a lower temperature the effect will be more pronounced.

Similar to the one dot case, one can extract information about the level spacing when one considers the current through the system at fixed bias tex2html_wrap_inline1320 while varying the gate voltage of one of the dots, a measurement first performed by van der Vaart et al. [12]. This is depicted in figure 12. The Coulomb repulsion energies and the level spacings are the same as before. The inelastic tunnelling coefficient is small compared to the dot-reservoir coupling. The empty levels are the levels that an excess electron can occupy. Note that no more than a single extra electron can be contained in the dot, since this is prevented by the Coulomb blockade. Since electrons carry a negative charge, a rise in the gate potential causes a downward shift of the energy levels.

The results are shown in figure 13 for a range of values of tex2html_wrap_inline1320. A few generic features can be noted which are also true for tunnelling through a single dot. Firstly, the current is periodic in the gate voltage with a period tex2html_wrap_inline1442. Only a single period is shown in the figure. Secondly, a significant current is only allowed to flow when the Coulomb blockade is overcome in both dots. This requires the lowest available level in each dot to lie within the energy window tex2html_wrap_inline1320. This is clearly shown in figure 13 where a larger bias voltage allows the current to flow at more values of the gate potential.

The most striking feature of figure 13 is the occurrence of sharp current peaks. These happen at values of the gate voltage where one of the occupied states of the first dot (containing the excess electron) lines up with an empty level in the second dot. It is clear that this will happen with a periodicity tex2html_wrap_inline1444 (in the figure tex2html_wrap_inline1462). When the bias voltage is such that several levels in the second dot are contained within the energy window tex2html_wrap_inline1320, then peaks will also occur at intervals tex2html_wrap_inline1466. This is the case in the third graph of figure 13, where tex2html_wrap_inline1468.

Finally, note that the current in the valleys between the peaks increases more or less linearly with the number of peaks. This reflects the fact that at a higher gate potential there are more electrons in the first dot which are able to tunnel downwards in energy into the second dot. Each tunnelling path has an associated off-resonance tunnelling rate of tex2html_wrap_inline1418 which will contribute an amount tex2html_wrap_inline1472 towards the total current (assuming tex2html_wrap_inline1474). Therefore the current minima should increase by this amount every time the gate potential is increased by an amount tex2html_wrap_inline1444.

This seems to be a much more powerful method for determining the single particle level spacing than the analogous experiment with a single dot. In the model used in this chapter, the line shape will be a multiple of the Bose-Einstein distribution. However, at very small energy separations tex2html_wrap_inline1396 the intrinsic width of the levels becomes significant and the lineshape will be approximately a Lorentzian of width tex2html_wrap_inline1480 near resonance but will be asymmetric off-resonance. This seems to corresponds at least qualitatively to recent experiment [12]. In the case of large tex2html_wrap_inline1482, the middle barrier is no longer the current limiting barrier and the current will not peak anymore but simply increase with tex2html_wrap_inline1396 until a saturation value of tex2html_wrap_inline1486 is reached. Further experiments will have to show whether it is justified to assume that the inelastic tunnelling rate can be approximated by the Bose-Einstein distribution. If this turns out to be a false assumption, then the master equation can still be used to model the effect of a more realistic inelastic tunnelling rate.


next up previous
Next: Conclusions Up: Tunnelling through two dots Previous: Ohmic conductance

Angus MacKinnon - Aonghus Mac Fhionghuin Fri Nov 8 18:10:54 gmt 1996