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Tunnelling through two dots in series

 

When studying the current and conductance properties of two quantum dots connected in series between the source and the drain, one obviously has to take into account the tunnelling between the dots. Inter-dot transitions are qualitatively different from transitions between a dot and a reservoir. The reservoir can be assumed to have a continuous density of states, so that electrons can always tunnel elastically into and out of the reservoir. Even though inelastic tunnelling events would in principle be allowed, their contribution would be relatively small compared to the elastic tunnelling rate. Therefore inelastic scattering only has a significant effect on the transport through a single dot if the scattering takes place inside the dot, i.e. relaxation.

As far as tunnelling between dots is concerned, it is clear that the elastic tunnelling rate is significant only when the energy levels in the dots line up. This is obviously not generally the case. Usually an electron would have to interact inelastically in order to tunnel to a different energy level in the neighbouring dot. The energy difference would normally be absorbed or provided by phonons.

As a theoretical model, one can consider the double dot system to be coupled to a phonon reservoir or a heat bath with a coupling strength tex2html_wrap_inline1330. The energy spectrum of the independent oscillators of the phonon reservoir is characterised by the density of phonon states tex2html_wrap_inline1332. Some work has been done to calculate the current through a double-barrier resonant structure with some interaction between electrons and photons [20, 21, 22]. The coupling to the optical phonons creates transmission subbands which are observable in the I-V characteristics. In this section, where inter-dot transmission is considered, the interaction with acoustic phonons will be the dominant mechanism. The energy spectrum for acoustic phonons is given by the Debye density of states.
equation291
In a two-dimensional electron gas the Debye temperature tex2html_wrap_inline1334 is approximately in the range tex2html_wrap_inline1336 [23]. This is of the order of a few tens of meV, which corresponds to several times the Coulomb interaction energy U. This is typically larger than the voltage drop across the device, so that one can simply use the phonon density of states below the cut-off energy tex2html_wrap_inline1342.

Phonons are bosons, so that the Pauli principle does not apply and states can be multiply occupied. The average occupation number of states at a given energy is given by the Bose-Einstein distribution tex2html_wrap_inline1344.
equation299
where tex2html_wrap_inline1346 is the Heaviside step function and E(-E) is the energy provided (absorbed) by the phonon bath. The Bose-Einstein distribution at positive and negative values of E differs by 1, which is indicative of the fact that a heat bath can always absorb energy.

Any plausible model for the inelastic tunnelling rate between the dots should take into account a Boltzmann factor, the density of states in the two dots and a term which describes the hybridisation between levels in adjacent dots. A simple model for the inelastic tunnelling rate tex2html_wrap_inline1356 between an energy level tex2html_wrap_inline1358 in the first dot and tex2html_wrap_inline1360 in the second dot is as follows
 equation304
where tex2html_wrap_inline1362 and tex2html_wrap_inline1364 are the densities of state for the energy levels. Considering the dots in isolation from the reservoirs, the eigenstates cannot be regarded as localised in each of the dots, but the wavefunctions will leak slightly into the other dot by virtue of the hopping potential tex2html_wrap_inline1366. This results in the overlap integrals tex2html_wrap_inline1368 and tex2html_wrap_inline1370. Naively this can be interpreted as the probability that the inelastic process can take place between the wavefunction components in the same dot. If a specific system is studied, then it is required to investigate the energy dependence of the off-diagonal elements of the Hamiltonian. However, here we are mostly concerned with generic features, so that the wavefunctions are calculated from a simple two-dimensional Hamiltonian with diagonal elements tex2html_wrap_inline1372 and tex2html_wrap_inline1374 and off-diagonal elements given by the constant hopping potential tex2html_wrap_inline1366. By calculating its eigenvectors the overlap matrix can be determined.
equation316
The above model is chosen for its relative simplicity, but it is expected to give results which are at least qualitatively correct. In principle, it is also possible to use this method using a more sophisticated model for the interdot tunnelling rate.

The density of states in the dots is broadened mainly as a result of the inelastic scattering, which is a prerequisite for the incoherent regime. To a first approximation the broadening can be considered as a Lorentzian distribution [24] with a broadening tex2html_wrap_inline1378 proportional to the phase-breaking rate. Now equation 29 can be rewritten as a single integral over the energy difference tex2html_wrap_inline1380 between the initial and final state.
equation323
with tex2html_wrap_inline1382.

It must be stressed that the broadening of the energy levels should be much less than the temperature. Otherwise it is not valid anymore to use the Boltzmann distribution to calculate the occupation probabilities. This assumption is consistent with the calculation of the reservoir-dot transition rate of section iii. Figure 6a shows the energy dependence of the inter-dot tunnelling rate for the case when the energy-levels are considered to be tex2html_wrap_inline1384-functions. However, it should still be taken into account that the level broadening is large compared to the coupling between the dots, causing the peaks in the transition rate at tex2html_wrap_inline1386 to be smeared. At energy differences tex2html_wrap_inline1388 which are small compared to the broadening, the transition rate can now be approximated by a Lorentzian of width tex2html_wrap_inline1390 and height tex2html_wrap_inline1392 (see figure 6b). At larger energy differences tex2html_wrap_inline1394 the function is sufficiently close to the Bose-Einstein distribution.

As the broadening is much smaller than the thermal energy, the inter-dot transition rate for small tex2html_wrap_inline1396 can get much larger than the transition rate between dot and reservoir so that the inter-dot transition is no longer the current-limiting process. In this case it is of no relevance whether the transition rate between the dots is infinite or simply very large. This suggests that the inter-dot transition rate may be approximated by the Bose-Einstein distribution tex2html_wrap_inline1398 at all values of tex2html_wrap_inline1396. This makes the mathematical analysis much more transparent.

When one calculates the transition rate between dots with a given occupation number, one should sum over all possible tunnelling events according to equation 8. The greatest contribution should come from the energy range where the electron can tunnel from levels which are mostly occupied to levels which are mostly empty. Outside this window the product tex2html_wrap_inline1402 falls off exponentially. However, since the Bose-Einstein distribution diverges at tex2html_wrap_inline1404, the total transition rate seems to be dominated by matching levels, even when they are situated at energies far removed from the Fermi level. This is clearly an unphysical situation. This anomaly can be removed by again including the broadening in the calculation of the transition rate. Alternatively, it can be argued that the transition rate for a given pair of levels is the combination of the previously defined rate and the rate at which electrons can get into an excited level. This second rate is the relaxation rate tex2html_wrap_inline1406. Remembering that the inverses of the rates of consecutive processes add together, the total inter-dot rate can be obtained for given occupation numbers.
equation347

In order to perform some realistic simulations it is helpful to know the dependence on the size of both the charging energy U and the confinement energy tex2html_wrap_inline1274. In the charging model approximation the Coulomb repulsion is inversely proportional to the capacitance C of the dot. This implies that the repulsion energy U is also inversely proportional to the area of the dot. The single particle energy level spacing is given by [25]
equation361
where tex2html_wrap_inline1416 is the effective mass of an electron in the two dimensional electron gas in which the quantum dot has been defined. It follows that both the Coulomb energy and the level spacing scale inversely proportionally to the area of the quantum dot.




next up previous
Next: Ohmic conductance Up: Incoherent tunnelling through two Previous: Tunnelling through a single

Angus MacKinnon - Aonghus Mac Fhionghuin Fri Nov 8 18:10:54 gmt 1996